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Returns: Error status Description: Determines how a path is to be displayed. Display types are:

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A number of MAO-free cocatalysts containing trimethylaluminum, TMA, have been studied Soga and coworkers21 23 prepared a number of catalytic systems Using supported zirconocene dichloride catalysts, productivities were close to those found for the simple solution systems Greater stereospeci city was achieved using bridged zirconocene systems, where the bridges included ethylenediindenyl systems, supported on alumina It is believed that the support enhances the profacial monomer selection by the Zr center and at the same time renders more favorable the beta-agostic interaction between it and the hydrogen atom on the beta-carbon atom of the growing chain The variation in results found for such systems is consistent with the need for precise structural control to achieve good polymerization and reproducible polymerization results The molecular weight distributions (MWD), Mw /Mn, for polyproplyene, PP, obtained from alumina supported catalysts are less than two.

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For ansa (meaning bent handle ) bridged systems, such as Et(THI)2ZrCl2, the polypropylene polymerization activities are only 10 20% those of the same zirconocene complexes in solution However, supported Cp2ZrCl2 catalysts exhibit productivities closer to those when the zirconocene is in solution Furthermore, the supported systems on alumina are more stereospeci c than corresponding soluble systems The supported symmetric zirconocenes give i-PP and s-PP with higher melting points and greater homosteric pentad populations It is believed that the supports enhance the profacial monomer selection by the Zr center and at the same time renders the beta-agostic interaction between it and atomic hydrogen on the beta carbon atom of the growing chain more favorable, as evidenced by a signi cantly lower molecular weight for the PP obtained with the heterogenized zirconocenes The molecular weight distributions of the alumina supported PP are less than 2.

Earlier, Kaminsky and Renner24 supported zirconocene derivatives on dehydroxylated silica and studied the polymerizatoin of propylene The catalysts had an activity of 1 104 g PP/mol Zr h This PP has a high stereoregularity and high melting point In solution, the same zirconocene catalyst has a much greater activity (4 106 g PP/mol Zr h) but the stereoregularity was less and the melting point of the PP lowed from 160 to 128 C Sacchi and coworkers25 found that even an aspeci c zirconocene catalyst can become isospeci c when bound Thus (Ind)2ZrCl2 in solution with MAO gave PP as a waxy product with an activity of 15 105 g PP/mol Zr h The PP had a [mm] = 018, [mr] = 046, and [rr] = 036 (m = meso; r = racemic).

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